Localization and Directionality of Surface Transport in Bi2Te3 Ordered 3D Nanonetworks

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2023Department
Ciencia de los Materiales e Ingeniería Metalúrgica y Química InorgánicaSource
ACS Nano - 2023, Vol. 17 n. 17 pp. 16960-16967Abstract
The resistance of an ordered 3D-Bi2Te3 nanowire nanonetwork was studied at low temperatures. Below 50 K the increase in resistance
was found to be compatible with the Anderson model for localization,
considering that conduction takes place in individual parallel channels
across the whole sample. Angle-dependent magnetoresistance measurements showed a distinctive weak antilocalization characteristic with a
double feature that we could associate with transport along two
perpendicular directions, dictated by the spatial arrangement of the
nanowires. The coherence length obtained from the Hikami−Larkin−
Nagaoka model was about 700 nm across transversal nanowires, which
corresponded to approximately 10 nanowire junctions. Along the individual
nanowires, the coherence length was greatly reduced to about 100 nm. The
observed localization effects could be the reason for the enhancement of the
Seebeck coefficient observed in the 3D-Bi2Te3 nanowire nanonetwork
compared to individual nanowires.
Subjects
metamaterials; bismuth telluride; 3D-AAO; nanonetwork; surface transport; localization effectsCollections
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