RT journal article
T1 Purcell Enhancement and Wavelength Shift of Emitted Light by CsPbI3 Perovskite Nanocrystals Coupled to Hyperbolic Metamaterials
A1 Pashaei Adl, Hamid
A1 Gorji, Setatira
A1 Karimi Habil, Mojtaba
A1 Suárez, Isaac
A1 Chirvony, Vladimir S.
A1 Gualdrón-Reyes, Andrés F.
A1 Mora-Seró, Iván
A1 Valencia, Luisa M.
A1 Mata Fernández, María de la
A1 Hernández-Saz, Jesús
A1 Molina Rubio, Sergio Ignacio
A1 Zapata Rodríguez, Carlos J.
A1 Martínez Pastor, Juan P.
A2 Ciencia de los Materiales e Ingeniería Metalúrgica y Química Inorgánica
K1 lead halide perovskites
K1 perovskite nanocrystals
K1 photonics
K1 hyperbolic metamaterials (HMMs)
K1 light-matter interaction
K1 Purcell factor
AB Manipulation of the exciton emission rate in nanocrystals of lead halide perovskites (LHPs) was demonstrated by means of coupling of excitons with a hyperbolic metamaterial (HMM) consisting of alternating thin metal (Ag) and dielectric (LiF) layers. Such a coupling is found to induce an increase of the exciton radiative recombination rate by more than a factor of three due to the Purcell effect when the distance between the quantum emitter and HMM is nominally as small as 10 nm, which coincides well with the results of our theoretical analysis. Besides, an effect of the coupling-induced long wavelength shift of the exciton emission spectrum is detected and modeled. These results can be of interest for quantum information applications of single emitters on the basis of perovskite nanocrystals with high photon emission rates.
PB AMER CHEMICAL SOC
SN 2330-4022
YR 2020
FD 2020-11
LK http://hdl.handle.net/10498/24159
UL http://hdl.handle.net/10498/24159
LA eng
DS Repositorio Institucional de la Universidad de Cádiz
RD 15-nov-2026