RT journal article T1 Chitin nanocrystals as bio-based adhesives for the development of sustainable cork composites A1 García Laynez, María del Carmen A1 Herrera Collado, Miriam A1 Molina Rubio, Sergio Ignacio A1 Sanz de León, Alberto A1 García Laynez, María del Carmen A2 Ciencia de los Materiales e Ingeniería Metalúrgica y Química Inorgánica K1 Chitin nanocrystals K1 Cork K1 Agrowaste valorization K1 Mechanical properties K1 Composites K1 Bio-based materials AB In this work, we demonstrate the potential of chitin nanocrystals (ChNCs), a sustainable and biobased nanomaterial, as an adhesive for valorizing cork waste and fabricating fully biobased composites through compression molding. SEM and XCT analyses confirmed that, when used at concentrations below 30 wt.%, ChNCs integrate homogeneously with cork by adhering uniformly to the cork cell walls, preserving its low density and inherent flexibility. Notably, composites containing 20 wt.% of ChNCs achieved superior mechanical properties (i.e. flexibility, strength and toughness) compared to composites with paraffin over a broad concentration range (5–70 wt.%). Unlike paraffin, which increases density by filling the cork cells, ChNCs maintain the porous structure while significantly enhancing compressive performance. These findings highlight the exceptional adhesive and reinforcing capabilities of ChNCs, paving the way for their use as a natural binder in developing sustainable cork composites and extending this approach to other agrowaste materials. PB Elsevier SN 2666-8939 YR 2025 FD 2025-03 LK http://hdl.handle.net/10498/37909 UL http://hdl.handle.net/10498/37909 LA eng DS Repositorio Institucional de la Universidad de Cádiz RD 21-sep-2026